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This paper is an attempt to explore the crucial roles of Information and Communication Technology (ICT) in management and provision of library services, and its implication to sustainable development in Nigeria. Despite the availability of wide opportunities offered by the advent of ICT, it has been observed that application of ICT to library services in Nigeria seems inadequate probably due to variety of challenges. With the methodology of simple literature review, the paper made effort to review related literature on ICT resources and ICT-based services in libraries, benefits of ICT and the role of library in sustainable development of Nigeria. The paper further identified the challenges of ICT application in libraries. It was recommended among others that, there should be improvement in the capacity and level of ICT adoption by libraries.