Date of this Version
APPLIED PHYSICS LETTERS 104 (2014)
Boron doped chromia (Cr2O3) thin films with substitutional doping levels between zero and 3% are grown using pulsed laser deposition in borane background gases. Magnetometry reveals a tunable increase in the Neel temperature of the (0001) textured Cr2BxO3-x thin films at a rate of about 10% with 1% oxygen site substitution preserving a net boundary magnetization. Spin resolved inverse photoemission measured after magnetoelectric annealing in subsequently reversed electric fields evidences voltage-controlled reversal of boundary magnetization and thus magnetoelectricity of Cr2BxO3-x. Conservation of magnetoelectricity far above room temperature makes ultra-low power voltage-controlled spintronic devices feasible.