Department of Chemistry
Date of this Version
3-8-1996
Abstract
We have investigated droplet nucleation and bubble cavitation in the quantum fluid helium-3 based on a nonlocal density-functional approach. A marked effect of droplet (or bubble) curvature on the rate of droplet nucleation or cavitation has been found. Without considering this curvature effect (as in the classical theory of nucleation) the droplet nucleation rate for helium-3 could be underestimated (i.e., near 1 K) or overestimated (i.e., near 2.5 K) by orders of magnitude, respectively; for bubble cavitation, the rate could be underestimated by more than twenty orders of magnitude (near 1 K).
Comments
Published by American Institute of Physics. J. Chem. Physics 104 (10), 8 March 1996. ©1996 American Institute of Physics. Permission to use. http://jcp.aip.org/.