Graduate Studies, UNL

 

Embargoed Master's Theses

First Advisor

Bai Cui

Second Advisor

Juan Macchi

Committee Members

Li Tan, Guillaume Hachet

Date of this Version

12-2025

Document Type

Thesis

Citation

A thesis presented to the faculty of the Graduate College at the University of Nebraska in partial fulfillment of requirements for the degree of Master of Science

Major: Mechanical Engineering and Applied Mechanics

Under the supervision of Professor Bai Cui

Lincoln, Nebraska, December 2025

Comments

Copyright 2025, Ryan A. Wall. Used by permission

Abstract

Hydrogen energy in the form of internal combustion engines [ICEs] dates to the invention of ICEs themselves. Current efforts to reduce carbon emissions of automobiles are highly invested in hydrogen ICEs, and so investigation into the materials needed for this application is highly important. One problem is hydrogen embrittlement.

Most metals fail through ductile fracture. Hydrogen embrittlement is characterized by a transition from ductile to brittle fracture. This transition results in a lower yield stress and a lack of warning before failure in the absence of significant elastic deformation. A cruicial step in this process is the dissociation of the H2 molecule into two H atoms, which dramatically lowers the size and allows diffusion through the matrix.

This project investigated a proprietary alloy used in engine valves for hydrogen ICEs. The alloy is a majority nickel with a high chromium content and lesser amounts of alloying elements such as titanium, aluminum, etc. A protective layer of CrN is present on the combustion surface. These valves were subjected to an intense exposure regimen in a high temperature hydrogen environment and then analyzed. Analysis includes SEM-EDS, TEM imaging and ACOM, micro- and nano-hardness, and Raman spectroscopy.

Advisor: Bai Cui

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