Department of Physics and Astronomy: Publications and Other Research

 

Evgeny Tsymbal Publications

ORCID IDs

Wang http://orcid.org/0000-0003-3146-5559

Paudel http://orcid.org/0000-0002-9952-9435

Suh http://orcid.org/0000-0002-0392-3391

Tsymbal http://orcid.org/0000-0002-6728-5480

Noh http://orcid.org/0000-0003-1905-2321

D. Lee http://orcid.org/0000-0002-0646-5226

Document Type

Article

Date of this Version

2020

Citation

Nature Communications (2020) 11: 2586

doi: 10.1038/s41467-020-16207-7

Supplementary material is available at https://doi.org/10.1038/s41467- 020-16207-7

Comments

Copyright 2020, the authors. Open access

License: CC BY 4.0 International

Abstract

Dielectrics have long been considered as unsuitable for pure electrical switches; under weak electric fields, they show extremely low conductivity, whereas under strong fields, they suffer from irreversible damage. Here, we show that flexoelectricity enables damage-free exposure of dielectrics to strong electric fields, leading to reversible switching between electrical states —insulating and conducting. Applying strain gradients with an atomic force microscope tip polarizes an ultrathin film of an archetypal dielectric SrTiO3 via flexoelectricity, which in turn generates non-destructive, strong electrostatic fields. When the applied strain gradient exceeds a certain value, SrTiO3 suddenly becomes highly conductive, yielding at least around a 108-fold decrease in room-temperature resistivity. We explain this phenomenon, which we call the colossal flexoresistance, based on the abrupt increase in the tunneling conductance of ultrathin SrTiO3 under strain gradients. Our work extends the scope of electrical control in solids, and inspires further exploration of dielectric responses to strong electromechanical fields.

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